Cloud Forming Potential of Aerosol from Light-duty Gasoline Direct Injection Vehicles
Advanced Search
Select up to three search categories and corresponding keywords using the fields to the right. Refer to the Help section for more detailed instructions.

Search our Collections & Repository

All these words:

For very narrow results

This exact word or phrase:

When looking for a specific result

Any of these words:

Best used for discovery & interchangable words

None of these words:

Recommended to be used in conjunction with other fields



Publication Date Range:


Document Data


Document Type:






Clear All

Add terms to the query box

Query box

Clear All

Cloud Forming Potential of Aerosol from Light-duty Gasoline Direct Injection Vehicles

Filetype[PDF-1.89 MB]

  • English

  • Details:

    • Resource Type:
    • Geographical Coverage:
    • Abstract:
      In this study, we evaluate the hygroscopicity and droplet kinetics of fresh and aged emissions from new generation gasoline direct injector engines retrofitted with a gasoline particulate filter (GPF). Furthermore, ageing and subsequent secondary aerosol formation is explored in (NH4)2SO4-seeded and non-seeded experiments. We explore the impacts on measured and predicted hygroscopicity, CCN-activity, and droplet kinetics of secondary aerosol mixed with initially insoluble carbonaceous materials versus very soluble (NH4)2SO4 seed. The chemical composition and density of the secondary aerosol (SA) formed from aging is measured with an HR-TOF-AMS and a custom-built APM-SMPS system. The supersaturated and subsaturated hygroscopicity of the fresh and aged emission is measured with a DMT Streamwise Thermal Gradient CCN counter and a hygroscopicity tandem differential mobility analyzer (HTDMA), respectively. The measurements show that the fresh gasoline emissions are only slightly hygroscopic in both supersaturated and subsaturated environments. Photochemical aging and subsequent condensation of the secondary aerosol formed from the co-emitted gas phase precursors increases the hygroscopicity of gasoline emissions. Without the GPF, both subsaturated and supersaturated hygroscopicity. When the engine was retrofitted with the GPF, the secondary aerosol (SA) experiments were seeded with (NH4)2SO4. In these experiments the presence of the condensing SA depresses the hygroscopicity of the salt-secondary aerosol mixture. The hygroscopicity was also depressed in the subsaturated regime with time. These changes in the hygroscopicity with aging were additionally sensitive to aerosol dry size distribution. We also used threshold droplet growth analysis (TDGA) to evaluate the effects of the condensing SA on droplet kinetics. These results have important implications for the assessment of cloud-aerosol indirect effects of salt-seeded and black carbonaceous aerosol cores. We concluded that in the new generation GDI vehicles the point of aerosol emissions will have significant influence on the impacts of the secondary and primary aerosols on climate.
    • Format:
    • Main Document Checksum:
    • File Type:

    Supporting Files

    • No Additional Files

    More +

    You May Also Like

    Checkout today's featured content at

    Version 3.18